Document of bibliographic reference 339492

BibliographicReference record

Type
Bibliographic resource
Type of document
Journal article
BibLvlCode
AS
Title
Towards understanding the characteristics of new particle formation in the Eastern Mediterranean
Abstract
To quantify the contribution of new particle formation (NPF) to ultrafine particle number and cloud condensation nuclei (CCN) budgets, one has to understand the mechanisms that govern NPF in different environments and its temporal extent. Here, we study NPF in Cyprus, an Eastern Mediterranean country located at the crossroads of three continents and affected by diverse air masses originating from continental, maritime, and desert-dust source areas. We performed 1-year continuous measurements of aerosol particles down to  1 nm in diameter for the first time in the Eastern Mediterranean and Middle East (EMME) region. These measurements were complemented with trace gas data, meteorological variables, and retroplume analysis. We show that NPF is a very frequent phenomenon at this site and has higher frequencies of occurrence during spring and autumn. NPF events were both of local and regional origin, and the local events occurred frequently during the month with the lowest NPF frequency. Some NPF events exhibited multiple onsets, while others exhibited apparent particle shrinkage in size. Additionally, NPF events were observed during the nighttime and during episodes of high desert-dust loadings. Particle formation rates and growth rates were comparable to those in urban environments, although our site is a rural one. Meteorological variables and trace gases played a role in explaining the intra-monthly variability of NPF events, but they did not explain why summer months had the least NPF frequency. Similarly, pre-existing aerosol loading did not explain the observed seasonality. The months with the least NPF frequency were associated with higher H2SO4 concentrations but lower NO2 concentrations, which is an indicator of anthropogenic influence. Air masses arriving from the Middle East were not observed during these months, which could suggest that precursor vapors important for nucleation and growth are transported to our site from the Middle East. Further comprehensive measurements of precursor vapors are required to prove this hypothesis.
WebOfScience code
https://www.webofscience.com/wos/woscc/full-record/WOS:000663965000005
Bibliographic citation
Baalbaki, R.; Pikridas, M.; Jokinen, T.; Laurila, T.; Dada, L.; Bezantakos, S.; Ahonen, L.; Neitola, K.; Maisser, A.; Bimenyimana, E.; Christodoulou, A.; Unga, F.; Savvides, C.; Lehtipalo, K.; Kangasluoma, J.; Biskos, G.; Petäjä, T.; Kerminen, V.-M.; Sciare, J.; Kulmala, M. (2021). Towards understanding the characteristics of new particle formation in the Eastern Mediterranean. Atmos. Chem. Phys. 21(11): 9223-9251. https://dx.doi.org/10.5194/acp-21-9223-2021
Topic
Marine
Is peer reviewed
true
Access rights
open access
Is accessible for free
true

Authors

author
Name
Rima Baalbaki
author
Name
Michael Pikridas
author
Name
Tuija Jokinen
author
Name
Tiia Laurila
author
Name
Lubna Dada
author
Name
Spyros Bezantakos
author
Name
Lauri Ahonen
author
Name
Kimmo Neitola
author
Name
Anne Maisser
author
Name
Elie Bimenyimana
author
Name
Aliki Christodoulou
author
Name
Florin Unga
author
Name
Chrysanthos Savvides
author
Name
Katrianne Lehtipalo
author
Name
Juha Kangasluoma
author
Name
George Biskos
author
Name
Tuukka Petäjä
author
Name
Veli-Matti Kerminen
author
Name
Jean Sciare
author
Name
Markku Kulmala

Links

referenced creativework
type
DOI
accessURL
https://dx.doi.org/10.5194/acp-21-9223-2021

Document metadata

date created
2021-07-01
date modified
2021-08-04