{"refrec":{"BRefID":382701,"RR":"<b>Chen, Y.Y.; Liu, S.; Zhu, L.; Seo, S.; Richter, A.; Li, X.C.; Ding, A.; Sun, W.F.; Shu, L.; Wang, X.; Valks, P.; Hendrick, F.; Koenig, T.K.; Volkamer, R.; Bai, B.; Wang, D.K.; Pu, D.C.; Sun, S.; Li, J.; Zuo, X.X.; Fu, W.T.; Li, Y.L.; Zhang, P.; Yang, X.; Fu, T.M.</b> (2023). Global observations of tropospheric Bromine monoxide (BrO) columns from TROPOMI. <i>JGR: Atmospheres 128(24)</i>: e2023JD039091. <a href=\"https://dx.doi.org/10.1029/2023JD039091\" target=\"_blank\">https://dx.doi.org/10.1029/2023JD039091</a>","BEntID":380442,"PublicFlag":1,"CheckedFlag":1,"wosflag":1,"vabbflag":1,"RefStringPartII":". <i>JGR: Atmospheres 128(24)</i>: e2023JD039091. <a href=\"https://dx.doi.org/10.1029/2023JD039091\" target=\"_blank\">https://dx.doi.org/10.1029/2023JD039091</a>","DocTypID":8,"DocType":"Journal article","MarineFlag":0,"FreshFlag":0,"BrackishFlag":0,"TerrestrialFlag":0,"Authorstring":"Chen, Y.Y.; Liu, S.; Zhu, L.; Seo, S.; Richter, A.; Li, X.C.; Ding, A.; Sun, W.F.; Shu, L.; Wang, X.; Valks, P.; Hendrick, F.; Koenig, T.K.; Volkamer, R.; Bai, B.; Wang, D.K.; Pu, D.C.; Sun, S.; Li, J.; Zuo, X.X.; Fu, W.T.; Li, Y.L.; Zhang, P.; Yang, X.; Fu, T.M.","OrigTitleTranslFlag":0,"Authorstringtrunc":"Chen, Y.Y. <i>et al.</i>","Englishabstract":"<p style=\"margin-left:0px;\">Bromine monoxide (BrO) plays an important role in tropospheric chemistry. The state-of-the-science TROPOspheric Monitoring Instrument (TROPOMI) offers the potential to monitor atmospheric composition with a fine spatial resolution of up to 5.5&nbsp;×&nbsp;3.5&nbsp;km<sup>2</sup>. We present here the retrieval of tropospheric BrO columns from TROPOMI. We implement a stratospheric correction scheme using a climatological approach based on the latest GEOS-Chem High Performance chemical transport model, and improve the tropospheric air mass factor calculation with TROPOMI surface albedo data accounting for the geometrical dependency. Our product presents a good level of consistency in comparison with measurements from ground-based zenith-sky differential optical absorption spectroscopy (<i>r</i>&nbsp;=&nbsp;0.67), aircrafts (<i>r</i>&nbsp;=&nbsp;0.46), and satellites (similar spatial distributions of BrO columns). Furthermore, our retrieval captures BrO enhancements in the polar springtime with values up to 7.8&nbsp;×&nbsp;10<sup>13</sup> molecules cm<sup>−2</sup> and identifies small-scale emission sources such as volcanoes and salt marshes. Based on TROPOMI data, we probe a blowing snow aerosol bromine mechanism in which the snow salinity is reduced to better match simulation and observation. Our TROPOMI tropospheric BrO product contributes high-resolution global information to studies investigating atmospheric bromine chemistry.","AbstractOtherLang":null,"BibLvlCode":"AS","StandardTitle":"Global observations of tropospheric Bromine monoxide (BrO) columns from TROPOMI","OrigTitleLangCode":"en","OrigTitleLangCodeExtended":"eng","OrigTitleLangID":15,"DateLastModified":{"date":"2026-04-22 01:32:37.467262","timezone_type":1,"timezone":"+02:00"},"UserAccessRight":null,"UserAccID":null,"AuthorKeywords":"TROPOMI; BrO; retrieval; GEOS-Chem","OtherDescriptors":null,"Notes":null,"AnaPub":2023,"MonPub":null,"DateUpdate":"2024-02-26","DateCreate":"2024-02-16","SecASFANote":null,"ConfID":null,"PeerRev":1,"VlizCoreFlag":1,"WoScode":"WOS:001138626900002","VABBcode":null,"OpenAcc":1,"DOI":"10.1029/2023JD039091"},"refs":null,"anarec":{"AnaID":382701,"PubliDate":2023,"Pagination":"e2023JD039091","XtraPublOfAnaID":null,"ISBN":null,"Volume":"128","Issue":"24","BRefMon":null,"BRefMonRR":null,"BRefXtra":null,"BRefXtraRR":null,"SerBRefID":272089,"SerRR":"Journal of Geophysical Research-Atmospheres. 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